Pt nanoparticle netlike-assembly as highly durable and highly active electrocatalyst for oxygen reduction reaction.

نویسندگان

  • Hong-Hui Wang
  • Zhi-You Zhou
  • Qiang Yuan
  • Na Tian
  • Shi-Gang Sun
چکیده

A Pt nanoparticle netlike-assembly (Pt-NNA) synthesized through a facile hydrothermal method, with high specific surface area and large overall size, exhibits much higher durability and 2.9 times higher mass activity for oxygen reduction reaction than commercial Pt black catalyst.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Synthesized Bimetallic Electrocatalyst for Oxygen Reduction Reaction in Polymer Electrolyte Fuel Cells

In the present study, a step by step process was applied to synthesize bimetallic electrocatalyst (Ru and Pt on VulcanXC-72R). This process can reduce the amount of platinum and increase the gas diffusion electrode (GDE) performance in the cathodic reaction of polymer electrolyte membrane fuel cells (PEMFCs). Using the impregnation by hydrothermal synthesis method, a series of electrocatalysts ...

متن کامل

Pt/C trapped in activated graphitic carbon layers as a highly durable electrocatalyst for the oxygen reduction reaction.

A thin nitrogen-doped graphitic carbon layer is elaborately introduced into the Pt/C surface to not only inhibit migration and dissolution of Pt nanoparticles, but also impart activity to the integral catalyst without blocking the inner Pt catalytic active sites. The corrosion of the carbon support can also be alleviated due to the outer graphitic coverage.

متن کامل

A simple preparation of very high methanol tolerant cathode electrocatalyst for direct methanol fuel cell based on polymer-coated carbon nanotube/platinum

The development of a durable and methanol tolerant electrocatalyst with a high oxygen reduction reaction activity is highly important for the cathode side of direct methanol fuel cells. Here, we describe a simple and novel methodology to fabricate a practically applicable electrocatalyst with a high methanol tolerance based on poly[2,2'-(2,6-pyridine)-5,5'-bibenzimidazole]-wrapped multi-walled ...

متن کامل

Synthesis of Supported Pt Alloy three Dimensional Rhombus Shapes Nanoparticles for Oxygen Reduction Reaction

In this study PtFeCo ternary alloys nanoparticles of three dimentional (3D) rhombus shapes dispersed on graphene nanosheets (PtFeCo/Gr) were successfully prepared and studied as electrocatalysts for oxygen reduction reaction (ORR) in polymer-electrolyte fuel cells. A combination of analytical techniques including powder X-ray diffraction, X-ray photoelectron spectra, inductively coupled plasma-...

متن کامل

High Pt Loading on Polydopamine Functionalized Graphene as a High Performance Cathode Electrocatalyst for Proton Exchange Membrane Fuel Cells

Morphology and size of platinum nanoparticles are a crucial factor in improving their catalytic activity and stability. Here, we firstly report the synthesis of high loading Pt nanoparticles on polydopamine reduced Graphene. The loading concentration of Pt (nanoparticles) NPs on Graphene can be adjusted in the range of 60-70%.With the insertion of polydopamine between Graphene oxide sheets, sta...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Chemical communications

دوره 47 12  شماره 

صفحات  -

تاریخ انتشار 2011